GB1064569A

GB1064569A – Oxidation process
– Google Patents

GB1064569A – Oxidation process
– Google Patents
Oxidation process

Info

Publication number
GB1064569A

GB1064569A
GB48305/64A
GB4830564A
GB1064569A
GB 1064569 A
GB1064569 A
GB 1064569A
GB 48305/64 A
GB48305/64 A
GB 48305/64A
GB 4830564 A
GB4830564 A
GB 4830564A
GB 1064569 A
GB1064569 A
GB 1064569A
Authority
GB
United Kingdom
Prior art keywords
gas
halide
metal
metal halide
oxygenating
Prior art date
1962-01-30
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)

Expired

Application number
GB48305/64A
Inventor
Alan Edward Comyns
Derek Howden
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)

British Titan Products Co Ltd

Original Assignee
British Titan Products Co Ltd
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
1962-01-30
Filing date
1964-11-27
Publication date
1967-04-05

Priority to NL288332D
priority
Critical
patent/NL288332A/xx

Priority to BE627783D
priority
patent/BE627783A/xx

Priority to NL134895D
priority
patent/NL134895C/xx

1962-01-30
Priority to GB3528/62A
priority
patent/GB991318A/en

1963-01-29
Priority to FR923086A
priority
patent/FR1355624A/en

1963-01-30
Priority to DEB70553A
priority
patent/DE1266278B/en

1963-01-30
Priority to FI630165A
priority
patent/FI42071C/en

1964-11-27
Priority to GB48305/64A
priority
patent/GB1064569A/en

1964-11-27
Application filed by British Titan Products Co Ltd
filed
Critical
British Titan Products Co Ltd

1965-11-22
Priority to FR39332A
priority
patent/FR89766E/en

1965-11-24
Priority to BE672781A
priority
patent/BE672781A/xx

1965-11-26
Priority to NL6515385A
priority
patent/NL6515385A/xx

1965-11-26
Priority to DEB84718A
priority
patent/DE1294938B/en

1965-11-26
Priority to NO160649A
priority
patent/NO120070B/no

1966-05-11
Priority to US549297A
priority
patent/US3463610A/en

1967-04-05
Publication of GB1064569A
publication
Critical
patent/GB1064569A/en

1969-07-02
Priority to US840598A
priority
patent/US3531247A/en

Status
Expired
legal-status
Critical
Current

Links

Espacenet

Global Dossier

Discuss

Classifications

C—CHEMISTRY; METALLURGY

C01—INORGANIC CHEMISTRY

C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C

C01B13/00—Oxygen; Ozone; Oxides or hydroxides in general

C01B13/14—Methods for preparing oxides or hydroxides in general

C01B13/20—Methods for preparing oxides or hydroxides in general by oxidation of elements in the gaseous state; by oxidation or hydrolysis of compounds in the gaseous state

C01B13/22—Methods for preparing oxides or hydroxides in general by oxidation of elements in the gaseous state; by oxidation or hydrolysis of compounds in the gaseous state of halides or oxyhalides

B—PERFORMING OPERATIONS; TRANSPORTING

B82—NANOTECHNOLOGY

B82Y—SPECIFIC USES OR APPLICATIONS OF NANOSTRUCTURES; MEASUREMENT OR ANALYSIS OF NANOSTRUCTURES; MANUFACTURE OR TREATMENT OF NANOSTRUCTURES

B82Y30/00—Nanotechnology for materials or surface science, e.g. nanocomposites

C—CHEMISTRY; METALLURGY

C01—INORGANIC CHEMISTRY

C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C

C01B13/00—Oxygen; Ozone; Oxides or hydroxides in general

C01B13/14—Methods for preparing oxides or hydroxides in general

C01B13/20—Methods for preparing oxides or hydroxides in general by oxidation of elements in the gaseous state; by oxidation or hydrolysis of compounds in the gaseous state

C01B13/22—Methods for preparing oxides or hydroxides in general by oxidation of elements in the gaseous state; by oxidation or hydrolysis of compounds in the gaseous state of halides or oxyhalides

C01B13/24—Methods for preparing oxides or hydroxides in general by oxidation of elements in the gaseous state; by oxidation or hydrolysis of compounds in the gaseous state of halides or oxyhalides in the presence of hot combustion gases

C—CHEMISTRY; METALLURGY

C01—INORGANIC CHEMISTRY

C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C

C01B13/00—Oxygen; Ozone; Oxides or hydroxides in general

C01B13/14—Methods for preparing oxides or hydroxides in general

C01B13/20—Methods for preparing oxides or hydroxides in general by oxidation of elements in the gaseous state; by oxidation or hydrolysis of compounds in the gaseous state

C01B13/22—Methods for preparing oxides or hydroxides in general by oxidation of elements in the gaseous state; by oxidation or hydrolysis of compounds in the gaseous state of halides or oxyhalides

C01B13/26—Methods for preparing oxides or hydroxides in general by oxidation of elements in the gaseous state; by oxidation or hydrolysis of compounds in the gaseous state of halides or oxyhalides in the presence of a fluidised bed

C—CHEMISTRY; METALLURGY

C01—INORGANIC CHEMISTRY

C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C

C01B13/00—Oxygen; Ozone; Oxides or hydroxides in general

C01B13/14—Methods for preparing oxides or hydroxides in general

C01B13/20—Methods for preparing oxides or hydroxides in general by oxidation of elements in the gaseous state; by oxidation or hydrolysis of compounds in the gaseous state

C01B13/22—Methods for preparing oxides or hydroxides in general by oxidation of elements in the gaseous state; by oxidation or hydrolysis of compounds in the gaseous state of halides or oxyhalides

C01B13/28—Methods for preparing oxides or hydroxides in general by oxidation of elements in the gaseous state; by oxidation or hydrolysis of compounds in the gaseous state of halides or oxyhalides using a plasma or an electric discharge

C—CHEMISTRY; METALLURGY

C01—INORGANIC CHEMISTRY

C01B—NON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C

C01B33/00—Silicon; Compounds thereof

C01B33/113—Silicon oxides; Hydrates thereof

C01B33/12—Silica; Hydrates thereof, e.g. lepidoic silicic acid

C01B33/18—Preparation of finely divided silica neither in sol nor in gel form; After-treatment thereof

C01B33/181—Preparation of finely divided silica neither in sol nor in gel form; After-treatment thereof by a dry process

C01B33/183—Preparation of finely divided silica neither in sol nor in gel form; After-treatment thereof by a dry process by oxidation or hydrolysis in the vapour phase of silicon compounds such as halides, trichlorosilane, monosilane

C—CHEMISTRY; METALLURGY

C01—INORGANIC CHEMISTRY

C01G—COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSES C01D OR C01F

C01G23/00—Compounds of titanium

C01G23/04—Oxides; Hydroxides

C01G23/047—Titanium dioxide

C01G23/07—Producing by vapour phase processes, e.g. halide oxidation

C—CHEMISTRY; METALLURGY

C01—INORGANIC CHEMISTRY

C01P—INDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS

C01P2004/00—Particle morphology

C01P2004/51—Particles with a specific particle size distribution

C—CHEMISTRY; METALLURGY

C01—INORGANIC CHEMISTRY

C01P—INDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS

C01P2004/00—Particle morphology

C01P2004/60—Particles characterised by their size

C01P2004/62—Submicrometer sized, i.e. from 0.1-1 micrometer

C—CHEMISTRY; METALLURGY

C01—INORGANIC CHEMISTRY

C01P—INDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS

C01P2004/00—Particle morphology

C01P2004/60—Particles characterised by their size

C01P2004/64—Nanometer sized, i.e. from 1-100 nanometer

C—CHEMISTRY; METALLURGY

C01—INORGANIC CHEMISTRY

C01P—INDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS

C01P2006/00—Physical properties of inorganic compounds

C01P2006/60—Optical properties, e.g. expressed in CIELAB-values

Abstract

Metal oxides are produced by forming a gas mixture containing a first metal halide, a first oxygenating gas and a fuel gas, the quantity of the latter being at least sufficient to maintain the temp. necessary for the oxidation of the metal halide, e.g. at least 600 DEG C. This mixture is burnt to produce a hot gas containing solid particles of metal oxide. This gas stream is passed into a reaction zone into which is introduced a second metal halide and a second oxygenating gas, at least one of these being introduced through a plurality of inlets, e.g. up to 20, spaced along the reaction zone in the direction of gas flow. The necessary temp. for oxidation of the second metal halide is maintained and the metal oxide produced is recovered. The first and second halide may form a white oxide and may be the same, e.g. chlorides of Ti, Al, Zr, Si. The first and second oxygenating gases may be the same, e.g. O2, or a free O2-containing gas, e.g. air or O2 enriched air. At least part of the second halide or oxygenating gas may be an unreacted excess of the first halide or oxygenating gas. The fuel gas may be CO or a hydrocarbon, e.g. C2H6, C3H8 or C4H10. The initial gas mixture may be preheated, e.g. to at least 150 DEG C., if the first metal halide is TiCl4 before being burnt. If the second metal halide is TiCl4 then the particulate metal oxide in the gas stream may have a mean size from 0.01 to 0.25 m . The ratio of first metal halide to fuel gas may be 1 : 2 to 4. The gas mixture may be burnt through a plurality of channels in a shaft furnace. The amount of metal oxide produced in the reaction zone may be from 1.01 to 10 times the total weight of metal oxide present in the gas stream. TiO2 produced preferably has a mean size of 0.15 to 0.35 m and may be formed with the addition of halides of Al, Si, Ce, Zr, and/or boron and/or water vapour and/or a subhalide of Ti and/or a source of K ions. The oxides formed from these additions may form a coating on the particles, especially if introduced after the second halide. Halogen liberated in the process may be recycled to produce further metal halide for use in the process.

GB48305/64A
1962-01-30
1964-11-27
Oxidation process

Expired

GB1064569A
(en)

Priority Applications (15)

Application Number
Priority Date
Filing Date
Title

NL288332D

NL288332A
(en)

1962-01-30

BE627783D

BE627783A
(en)

1962-01-30

NL134895D

NL134895C
(en)

1962-01-30

GB3528/62A

GB991318A
(en)

1962-01-30
1962-01-30
Finely divided metal oxides

FR923086A

FR1355624A
(en)

1962-01-30
1963-01-29

New process for the production of finely divided metal oxides and oxides obtained

FI630165A

FI42071C
(en)

1962-01-30
1963-01-30

Method for the production of fine titanium, zirconium or alumina oxides

DEB70553A

DE1266278B
(en)

1962-01-30
1963-01-30

Process for the production of finely divided metal oxides by the oxidation of metal halides

GB48305/64A

GB1064569A
(en)

1962-01-30
1964-11-27
Oxidation process

FR39332A

FR89766E
(en)

1962-01-30
1965-11-22

New process for the production of finely divided metal oxides and oxides obtained

BE672781A

BE672781A
(en)

1962-01-30
1965-11-24

NL6515385A

NL6515385A
(en)

1962-01-30
1965-11-26

DEB84718A

DE1294938B
(en)

1962-01-30
1965-11-26

Process for the production of finely divided metal oxides

NO160649A

NO120070B
(en)

1962-01-30
1965-11-26

US549297A

US3463610A
(en)

1962-01-30
1966-05-11
Process for the production of particulate titanium dioxide

US840598A

US3531247A
(en)

1962-01-30
1969-07-02
Process for the production of finely-divided metal oxides by multiple oxidation

Applications Claiming Priority (2)

Application Number
Priority Date
Filing Date
Title

GB3528/62A

GB991318A
(en)

1962-01-30
1962-01-30
Finely divided metal oxides

GB48305/64A

GB1064569A
(en)

1962-01-30
1964-11-27
Oxidation process

Publications (1)

Publication Number
Publication Date

GB1064569A
true

GB1064569A
(en)

1967-04-05

Family
ID=26238381
Family Applications (2)

Application Number
Title
Priority Date
Filing Date

GB3528/62A
Expired

GB991318A
(en)

1962-01-30
1962-01-30
Finely divided metal oxides

GB48305/64A
Expired

GB1064569A
(en)

1962-01-30
1964-11-27
Oxidation process

Family Applications Before (1)

Application Number
Title
Priority Date
Filing Date

GB3528/62A
Expired

GB991318A
(en)

1962-01-30
1962-01-30
Finely divided metal oxides

Country Status (8)

Country
Link

US
(2)

US3463610A
(en)

BE
(2)

BE672781A
(en)

DE
(2)

DE1266278B
(en)

FI
(1)

FI42071C
(en)

FR
(2)

FR1355624A
(en)

GB
(2)

GB991318A
(en)

NL
(3)

NL6515385A
(en)

NO
(1)

NO120070B
(en)

Cited By (4)

* Cited by examiner, † Cited by third party

Publication number
Priority date
Publication date
Assignee
Title

US5599519A
(en)

*

1992-08-10
1997-02-04
Tioxide Group Services Limited
Oxidation of titanium tetrachloride to form titanium dioxide

US6207131B1
(en)

1996-07-25
2001-03-27
Kerr-Mcgee Chemical Llc
Method and apparatus for producing titanium dioxide

USRE39068E1
(en)

*

1996-07-25
2006-04-18
Magyar John C
Method and apparatus for producing titanium dioxide

DE102007049296A1
(en)

2007-10-12
2009-04-16
Kronos International, Inc.

Multi-stage process for the production of titanium dioxide

Families Citing this family (8)

* Cited by examiner, † Cited by third party

Publication number
Priority date
Publication date
Assignee
Title

US4012201A
(en)

*

1973-03-22
1977-03-15
Tioxide Group Limited
Reactor

GB1429333A
(en)

*

1973-03-22
1976-03-24
British Titan Ltd
Reactor

IN152047B
(en)

*

1978-12-04
1983-10-01
Du Pont

IT1130853B
(en)

*

1980-01-11
1986-06-18
Montedison Spa

POST-TREATED TITANIUM DIOXIDE AND PROCEDURE TO OBTAIN IT

US4803056A
(en)

*

1983-07-22
1989-02-07
Kerr-Mcgee Chemical Corporation
System for increasing the capacity of a titanium dioxide producing process

US5562764A
(en)

*

1994-06-28
1996-10-08
E. I. Du Pont De Nemours And Company
Process for preparing improved TIO2 by silicon halide addition

DE69900507T2
(en)

*

1998-05-27
2002-06-06
Du Pont

CONTROLLING PARTICLE SIZE IN PYROHYDROLYSIS OF METAL CHLORIDES

US6387347B1
(en)

*

2000-02-14
2002-05-14
Millennium Inorganic Chemicals, Inc.
Controlled vapor phase oxidation of titanium tetrachloride to manufacture titanium dioxide

Family Cites Families (6)

* Cited by examiner, † Cited by third party

Publication number
Priority date
Publication date
Assignee
Title

US2964386A
(en)

*

1958-03-06
1960-12-13
British Titan Products
Preparation of titanium dioxide

FR1231998A
(en)

*

1958-07-30
1960-10-04
British Titan Products

Process for preparing titanium dioxide

US3068113A
(en)

*

1960-06-21
1962-12-11
Pittsburgh Plate Glass Co
Method of preparing metal oxides

US3147077A
(en)

*

1960-06-24
1964-09-01
British Titan Products
Production of titanium dioxide

US3078148A
(en)

*

1961-05-26
1963-02-19
Cabot Corp
Process for making titanium dioxide

US3275411A
(en)

*

1963-04-08
1966-09-27
American Cyanamid Co
Plasma production of titanium dioxide

0

NL
NL288332D
patent/NL288332A/xx
unknown

BE
BE627783D
patent/BE627783A/xx
unknown

NL
NL134895D
patent/NL134895C/xx
active

1962

1962-01-30
GB
GB3528/62A
patent/GB991318A/en
not_active
Expired

1963

1963-01-29
FR
FR923086A
patent/FR1355624A/en
not_active
Expired

1963-01-30
DE
DEB70553A
patent/DE1266278B/en
active
Pending

1963-01-30
FI
FI630165A
patent/FI42071C/en
active

1964

1964-11-27
GB
GB48305/64A
patent/GB1064569A/en
not_active
Expired

1965

1965-11-22
FR
FR39332A
patent/FR89766E/en
not_active
Expired

1965-11-24
BE
BE672781A
patent/BE672781A/xx
unknown

1965-11-26
NO
NO160649A
patent/NO120070B/no
unknown

1965-11-26
NL
NL6515385A
patent/NL6515385A/xx
unknown

1965-11-26
DE
DEB84718A
patent/DE1294938B/en
active
Pending

1966

1966-05-11
US
US549297A
patent/US3463610A/en
not_active
Expired – Lifetime

1969

1969-07-02
US
US840598A
patent/US3531247A/en
not_active
Expired – Lifetime

Cited By (5)

* Cited by examiner, † Cited by third party

Publication number
Priority date
Publication date
Assignee
Title

US5599519A
(en)

*

1992-08-10
1997-02-04
Tioxide Group Services Limited
Oxidation of titanium tetrachloride to form titanium dioxide

US6207131B1
(en)

1996-07-25
2001-03-27
Kerr-Mcgee Chemical Llc
Method and apparatus for producing titanium dioxide

USRE39068E1
(en)

*

1996-07-25
2006-04-18
Magyar John C
Method and apparatus for producing titanium dioxide

DE102007049296A1
(en)

2007-10-12
2009-04-16
Kronos International, Inc.

Multi-stage process for the production of titanium dioxide

US8114376B2
(en)

2007-10-12
2012-02-14
Kronos International, Inc.
Multistage method for manufacturing titanium dioxide

Also Published As

Publication number
Publication date

BE627783A
(en)

GB991318A
(en)

1965-05-05

NL134895C
(en)

NO120070B
(en)

1970-08-24

FR89766E
(en)

1967-08-18

US3463610A
(en)

1969-08-26

FR1355624A
(en)

1964-03-20

DE1266278B
(en)

1968-04-18

NL6515385A
(en)

1966-05-31

BE672781A
(en)

1966-05-24

NL288332A
(en)

FI42071B
(en)

1970-02-02

DE1294938B
(en)

1969-05-14

US3531247A
(en)

1970-09-29

FI42071C
(en)

1970-05-11

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(en)

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